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Charge dynamics in the half-metallic ferromagnet CrO_2

by: EJ Singley, CP Weber, DN Basov, A Barry, JMD Coey
Physical Review B, Vol. 60, No. 6. (1999), 4126.


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Infrared spectroscopy is used to investigate the electronic structure and charge carrier relaxation in crystalline films of CrO 2 which is the simplest of all half-metallic ferromagnets. Chromium dioxide is a bad metal at room temperature but it has a remarkably low residual resistivity ( < 5 μΩ cm) despite the small spectral weight associated with free carrier absorption. The infrared measurements show that low residual resistivity is due to the collapse of the scattering rate at ω < 2000 cm -1 . The blocking of the relaxation channels at low ω and T can be attributed to the unique electronic structure of a half-metallic ferromagnet. In contrast to other ferromagnetic oxides; the intraband spectral weight is constant below the Curie temperature.


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